Nuclear Physics and Atomic Energy

ßäåðíà ô³çèêà òà åíåðãåòèêà
Nuclear Physics and Atomic Energy

  ISSN: 1818-331X (Print), 2074-0565 (Online)
  Publisher: Institute for Nuclear Research of the National Academy of Sciences of Ukraine
  Languages: Ukrainian, English
  Periodicity: 4 times per year

  Open access peer reviewed journal


 Home page   About 
Nucl. Phys. At. Energy 2026, volume 27, issue 2, pages 142-147.
Section: Nuclear Physics.
Received: 17.03.2026; Accepted: 25.05.2026; Published online: 25.06.2026.
PDF Full text (en)
https://doi.org/10.15407/jnpae2026.02.142

Determination of absolute probabilities of low-intensity gamma ray emission during the decay of 235U for the purposes of nuclear forensics

O. Zhukov1, V. Lebed1,2, I. Maliuk1, M. Strilchuk1,*, V. Tryshyn1

1 Institute for Nuclear Research, National Academy of Sciences of Ukraine, Kyiv, Ukraine
2 Taras Shevchenko National University of Kyiv, Kyiv, Ukraine


*Corresponding author. E-mail address: myst@meta.ua

Abstract: The value of absolute emission probabilities from the decay of 235U in the energy range of 200-450 keV was refined by using semiconductor gamma spectrometry with a reference material containing highly enriched uranium and mathematical modelling of the measurement geometry. This refinement is essential for the accurate gamma-spectrometric determination of characteristics (signatures) of highly enriched uranium that are crucial for nuclear forensics, such as model age and 228Th impurity. This clarification is also useful from the point of view of fundamental nuclear physics, as it introduces significant changes in the data concerning the 231Th level scheme from the alpha decay of 235U.

Keywords: 235U, nuclear forensics, highly enriched uranium, model age, gamma spectrometry, absolute emission probability.

References:

1. FRAM Plutonium and Uranium Isotopic Analysis. Application Software. https://www.ortec-online.com/products/software/fram

2. X-5 Monte Carlo Team. MCNP - A General Monte Carlo N-Particle Transport Code. Version 5. Vol. I. Overview and Theory. LA-UR-03-1987 (Los Alamos, Los Alamos National Laboratory, 2005) 340 p. https://mcnp-green.lanl.gov/pdf_files/TechReport_2003_LANL_LA-UR-03-1987Revised212008_SweezyBoothEtAl.pdf

3. S. Agostinelli et al. Geant4 - a simulation toolkit. Nucl. Instrum. Methods A 506(3) (2003) 250. https://doi.org/10.1016/S0168-9002(03)01368-8

4. R.B. Firestone, V.S. Shirley. Table of Isotopes. 8th ed. (New York, John Wiley & Sons, 1996) 2877 p. https://openlibrary.org/books/OL809633M/Table_of_isotopes?utm_source=chatgpt.com

5. A. Luca, M. A. Kellett. A new evaluation of the nuclear decay data of 223Ra. EPJ Web Conf. 239 (2020) 23002. https://doi.org/10.1051/epjconf/202023923002

6. M. Strilchuk. WinSpectrum v3.24. User manual.

7. E. Browne, J.K. Tuli. Nuclear Data Sheets for A = 231. Nucl. Data Sheets 114 (2013) 751. https://doi.org/10.1016/j.nds.2013.05.002

8. B. Singh et al. Nuclear Data Sheets for A = 219. Nucl. Data Sheets 175 (2021) 150. https://doi.org/10.1016/J.NDS.2021.06.002

9. B. Singh et al. Nuclear Data Sheets for A = 211. Nucl. Data Sheets 114 (2013) 661. https://doi.org/10.1016/j.nds.2013.05.001

10. B. Singh, J.K. Tuli, E. Browne. Nuclear Structure and Decay Data for A = 231 Isobars. Nucl. Data Sheets 185 (2022) 560. https://doi.org/10.1016/j.nds.2022.10.002

11. M.-C. Lépy et al. Photon emission intensities in the decay of U-235. Appl. Radiat. Isot. 126 (2017) 150. https://doi.org/10.1016/j.apradiso.2016.12.045

12. M. Marouli et al. Measurement of absolute γ-ray emission probabilities in the decay of 235U. Appl. Radiat. Isot. 132 (2018) 72. https://doi.org/10.1016/j.apradiso.2017.10.049

13. F.A. Danevich et al. Emission intensities of gamma transitions in 235U alpha decay. Eur. Phys. J. A 61 (2025) 264. https://doi.org/10.1140/epja/s10050-025-01746-8